Development and characterization of enriched bioplastics made from whole seaweed and carrageenan for food packaging

Eunice Lua Hanry1 and Noumie Surugau1

1Seaweed Research Unit, Faculty of Science and Natural Resources, Universiti Malaysia Sabah,

88400 Kota Kinabalu, Sabah, Malaysia

 

Recently, seaweed and its hydrocolloids were being promoted as ingredient for biodegradable plastics.  In this study, bioplastics were developed from whole seaweed (Kappaphycus

alvarezii) biomass (WS), semi-refined carrageenan (SRC) and refined carrageenan (RC). To enhance their properties, they were dyed using butterfly pea flower (Clitoria ternatea L.),

bougainvillea flower; and dragon fruit (Hylocereus polyrhizus) peel extracts. The bioplastics

development employed material-to-water ratio of 1:50; 2% (v/v) glycerol as plasticizer and 5% (v/v) natural dye. As results, the bioplastics were 0.03 – 0.100 mm in thickness which is in the

range of commercial food packaging.  Without dye, the WS, SRC and RC bioplastics has opacity (mm-1) of 4.14 ± 0.45, 3.50 ± 0.30 and 1.63 ± 0.31, respectively; meanwhile colour

difference (∆E) were 29.6 ± 0.1, 14.2 ± 0.1 and 6.4 ± 0.1, respectively. RC bioplastic has the highest tensile strength (12.80 ± 0.90 MPa) and elongation-at-break (25.7 ± 0.5 %), followed

by SRC (8.0 ± 0.4 MPa, 21.3 ± 0.6%) and WS (5.4 ± 0.7 MPa, 17.9 ± 1.0 %). No significant difference in water vapour permeability (WVP); WS degraded the fastest with all bioplastics

fully degraded after 18 days; and shelf life (at 25oC, 56% RH) up to 17 weeks. For the dyed bioplastics, the natural dye blended well into the natural colour of base material resulting in

attractive shade. Mechanical properties, WVP and biodegradability were not significantly affected but shelf-life was 20 – 30% longer. Seaweed bioplastics have a potential as green

alternative for single-use non-degradable food packaging.